April 25, 2024

When Light and Electrons Spin Together: Advancing Toward Petahertz Electronics Based on Quantum Materials

An infrared pulse (blue) thrills the electron dynamics wholesale Na3Bi. Due to strong spin-orbit coupling, the spin-up electrons (red arrow) and spin-down electrons (blue arrow) follow various motion, which can be tracked by the emitted harmonic light (blue and violet pulses). Credit: © Nicolas Tancogne-Dejean/ Jörg Harms, MPSD
Theoretical physicists at the Max Planck Institute for the Structure and Dynamics of Matter (MPSD) have shown how the coupling between extreme lasers, the motion of electrons, and their spin affects the emission of light on the ultrafast timescale.
Electrons, which exist in all type of matter, are charged particles and for that reason respond to the application of light. When an extreme light field strikes a solid, electrons experience a force, called the Lorentz force, that drives them and induces some splendid dynamics showing the residential or commercial properties of the material. This, in turn, leads to the emission of light by the electrons at numerous wavelengths, a widely known phenomenon called high-harmonic generation.
Exactly how the electrons move under the influence of the light field depends on a complicated mixture of homes of the solid, including its balances, geography, and band structure, along with the nature of the light pulse. Additionally, electrons are like spinning tops. They have a propensity to rotate either clockwise or counter-clockwise, a residential or commercial property called the “spin” of the electrons in quantum mechanics.

In a current research study, a group from the MPSD carried out the tough job of understanding how the light and the spin of the electron can communicate in Na3Bi, a topological material referred to as a Dirac semimetal (the three-dimensional analog of graphene), through a result referred to as spin-orbit coupling. This relativistic effect couples the particles spin to its motion inside a possible, a potential that intense light can modify on the ultrafast timescale.
A better understanding of how spin-orbit coupling influences the electron characteristics on these timescales is an important step towards comprehending the electron characteristics in complex quantum materials, where this result is frequently present. Undoubtedly, it is the spin-orbit coupling that often makes quantum products intriguing for future technological applications. It is anticipated to lead to the next generation of electronic devices, particularly topological electronic systems.
The authors show how spin-orbit coupling affects the velocity of the electrons within the electron bands of solids, efficiently imitating a magnetic field that depends on the electrons spin.
They show how modifications in the electron speed can affect the electron dynamics in Na3Bi which this impact can often be damaging to the generation of high-order harmonics. While this material is non-magnetic, the group has shown that the spin of the electrons is essential for the characteristics, as it combines to the possible felt by the electrons, which is customized by the intense used light-field.
These changes include essential information of the internal electron characteristics. Given that it is currently challenging to measure spin currents, the present work opens up fascinating point of views towards utilizing extreme light to perform high-harmonic spectroscopy of spin currents, as well as magnetization characteristics, or uncommon spin textures that can be present in quantum products.
This work serves as a platform for a better understanding of the link between spin-orbit coupling, spin existing, geography, and electron dynamics in solids driven by strong fields– an essential step towards the advancement of petahertz electronic devices based on quantum products.
Recommendation: “Effect of spin-orbit coupling on the high harmonics from the topological Dirac semimetal Na3Bi” by Nicolas Tancogne-Dejean, Florian G. Eich and Angel Rubio, 6 July 2022, npj Computational Materials.DOI: 10.1038/ s41524-022-00831-6.

Due to strong spin-orbit coupling, the spin-up electrons (red arrow) and spin-down electrons (blue arrow) follow different movement, which can be tracked by the discharged harmonic light (blue and violet pulses). When an intense light field hits a strong, electrons experience a force, called the Lorentz force, that drives them and causes some beautiful dynamics showing the properties of the material. Exactly how the electrons move under the influence of the light field depends on a complicated mixture of residential or commercial properties of the strong, including its symmetries, geography, and band structure, as well as the nature of the light pulse. A much better understanding of how spin-orbit coupling influences the electron characteristics on these timescales is a crucial step towards comprehending the electron characteristics in intricate quantum materials, where this effect is typically present.