May 2, 2024

Ultrafast Magnetism: Intense Lasers Magnetize Solids Within Attoseconds

An extreme laser pulse is shone onto the material, causing ultrafast spin flipping processes that occur on a timescale of ~ 100 attoseconds. Credit: © J. Harms, MPSD
Intense laser light can develop attosecond magnetism in solids with heavy atoms, offering brand-new insights into magnetization and potentially making it possible for ultrafast memory devices.
Intense laser light can cause magnetism in solids on the attosecond scale– the fastest magnetic reaction to date. That is the finding reached by theoreticians at the MPSD, who used sophisticated simulations to investigate the magnetization procedure in numerous 2D and 3D products. Their computations show that, in structures with heavy atoms, the fast electron dynamics initiated by the laser pulses can be converted to attosecond magnetism. The work has actually been released in the journal npj Computational Materials.
The team focused on several benchmark 2D and 3D product systems, however the results use to all materials that include heavy atomic constituents. “The heavy atoms are particularly essential, because they cause a strong spin-orbit interaction,” discusses lead author Ofer Neufeld. “This interaction is essential to converting the light-induced electron motion into spin polarization– to put it simply, into magnetism. Otherwise, light just does not engage with the electrons spin.”

Intense laser light can induce magnetism in solids on the attosecond scale– the fastest magnetic response to date. Their computations reveal that, in structures with heavy atoms, the quick electron characteristics initiated by the laser pulses can be converted to attosecond magnetism. Each electrons spin instructions depends on the chemical environment around it, for instance, which atoms it can see and where other electrons are. All of a sudden, their simulations revealed that these particularly powerful lasers do magnetize products, even though the magnetism is short-term– it lasts just until the laser pulse is turned off. The laser successfully accelerates the electrons in circular-like orbits in the space of a few hundred attoseconds.

Much like small compass needles, electrons can also be thought of as having an internal needle that indicates some instructions in area, e.g. up or down– the so-called spin. Each electrons spin instructions depends on the chemical environment around it, for example, which atoms it can see and where other electrons are. In non-magnetic materials, the electrons spin similarly in all instructions. In contrast, when the private electrons spins line up with each other to point in the same direction, the product becomes magnetic.
The theoreticians set out to examine what magnetic phenomena can occur when solids communicate with extreme linearly-polarized laser pulses, that generally speed up electrons on very quick timescales inside matter. “These conditions are interesting to explore, due to the fact that when the laser pulses have a linear polarization, they are normally thought not to induce any magnetism,” says Neufeld.
Unexpectedly, their simulations showed that these especially powerful lasers do magnetize materials, even though the magnetism is transient– it lasts only up until the laser pulse is turned off. The most impressive finding, nevertheless, worried the speed of this procedure: The magnetization develops on extremely short timescales, less than 500 attoseconds– a prediction for the fastest magnetic action ever.
Utilizing advanced simulation tools to explain the underlying system, the group showed that the intense light flips the electrons spins backward and forward. The laser successfully speeds up the electrons in circular-like orbits in the space of a few hundred attoseconds. These strong spin-orbit interactions then align the spin directions. The procedure can be envisioned as a bowling ball moving throughout a surface area which then begins to roll: In this analogy, the light pushes the ball around, and the spin-orbit interactions (a force emerging from the nearby heavy nuclei as the electron orbits around it) trigger it to roll back and forth, magnetizing it. Both forces act together to get the ball rolling.
The results offer fascinating new insights into the principles of magnetization, states Neufeld: “We discovered that its an extremely nonlinear result which can be tuned by the lasers residential or commercial properties. The outcomes hint, though do not unequivocally show, that the ultimate speed limit for magnetism is a number of tens of attoseconds, since thats the natural speed limit of electronic movement.”
Understanding these light-induced magnetization procedures at their basic level in a variety of materials is a crucial step towards the development of ultrafast memory devices and changes the present understanding of magnetism.
Referral: “Attosecond magnetization dynamics in non-magnetic materials driven by intense femtosecond lasers” by Ofer Neufeld, Nicolas Tancogne-Dejean, Umberto De Giovannini, Hannes Hübener and Angel Rubio, 23 March 2023, npj Computational Materials.DOI: 10.1038/ s41524-023-00997-7.